H2020-lce-2014-1 New knowledge and technologies research & innovation actions
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H2020-LCE-2014-1 New knowledge and technologies RESEARCH & INNOVATION ACTIONS
Deliverable 6.3 Dissemination Workshop 1 Proposal acronym: SWInG Proposal number: SEP-210184411 Duration: 36 months Name of the coordinating person: Dr. Marc Meuris, Interuniversitair Micro-Elektronica Centrum, Belgium Participant Participant legal name Country Organisation 1 (Coord.) Interuniversitair Micro-Elektronica Centrum (imec) Belgium Research institute 2 Nederlandse Organisatie voor toegepast- natuurwetenschappelijk onderzoek (TNO) Netherlands Research institute 3 Helmholtz-Zentrum Berlin für Materialien und Energie (HZB) Germany
Research institute 4 Zentrum für Sonnenenergie- und Wasserstoff- Forschung Baden-Württemberg (ZSW) Germany
Research institute 5 CNRS-Institut des Matériaux Jean Rouxel (IMN) France Research institute 6 Universiteit Gent (UG) Belgium University 8 Midsummer AB (MS) Sweden SME
Ref. Ares(2016)6791972 - 05/12/2016 2
During the first project-year, the SWInG consortium was selected to organize the 7 th European Kesterite Workshop. This Workshop aimed to provide a forum to stimulate discussion on current issues to improve understanding of Kesterites. Therefore, only a compact audience (80 people) with a focus on important and unpublished results was allowed to participate, this to keep its valued open character. These 80 attendants were coming from 30 institutes: CEA-Liten, Crystalsol, Çukurova Univ., DTU, Empa, ENEA, Ghent Univ., HZB, Imec, IMN, IMRA, Imperial CL, IREC, KIT, Max- Planck Institute, Northumbria Univ., SAS, TNO, TTU, Univ. of Grenoble, Univ. of Hasselt, Univ. of Jena, Univ. of Leuven, Univ. of Madrid, Univ. of Oldenburg, Univ. of Oslo, Univ. of Strathclyde, UNSW, Uppsala Univ., and ZSW. A Ph.D. student pre-meeting Workshop was organised on the 16 th of November 2016, at the High Tech Campus in Eindhoven, the Netherlands. This meeting was completely student organised and allow participating Ph.D. students (30 people) to present and discuss Kesterite-related topics and results among themselves. The actual Kesterite Workshop was held from 17 th to 18
th of November 2016 in Leuven, Belgium, at Imec's premises. It was an inspiring meeting to discuss the latest results, current problems and future needs with regards to Kesterite materials and solar cells. A table listing all 7 Kesterite Workshops, the scientific program of the 7 th European Kesterite Workshop, and a few pictures are given below.
PLACE ORGANIZER ATTENDANTS 1 2010 Uppsala, Sweden UU-ÅSC
25 2 2011 Barcelona, Spain IREC
65 3 2012 Luxembourg, Luxembourg ULUX
100 4 2013 Berlin, Germany HZB
80 5 2014 Tallinn, Estonia TUT
80 6 2015 Newcastle, UK NU 80 7 2016
Leuven, Belguim IMEC
80 3
th 08:30 Registration Welcome coffee Imec 5, 0 th floor: Lobby Imec 5, 1 st floor: Lounge 09:15 Opening session Chair = Jes Larsen, Uppsala University Imec 5, 2 nd floor: Room 2A 09:15 Welcome Speech by Jo De Boeck and Bart Vermang, imec
Session 1 – Impact of Ge on absorber formation
09:35 – Different pathways to solution-processed CZGSSe absorbers for thin-film solar cells, by Thomas Schnabel, ZSW
09:55 – Understanding the positive role of Ge in CZTSe:Ge solar cells, by Sergio Giraldo, IREC
10:15 – Fabrication and characterization of 4.2 % efficient CZGSe based solar cells, by Guy Brammertz, imec
Imec 5: Lounge 11:05 Session 2 – Kesterite absorber optimization Chair = Susan Schorr, HZB Imec 5: Room 2A 11:05 – Substitution of Li for Cu in CZTSe: toward wide band gap absorber with low cation-disorder for thin film solar cells, by Alain Lafond, IMN
11:25 – Alkali doping in solution processed kesterite solar cells, by Stefan
11:45 – Beyond 10 % efficient sulfide kesterite CZCTS solar cell: role of cadmium alloying, by Chang Yan, UNSW
12:05 – Influence of SnS secondary phase on CZTS Solar cells, by Yi Ren, Uppsala University
Imec 5: Lounge
Imec 5: Room 2A 13:25 – Study on the tetragonal distortion (c/2a) of CZTSe absorbers, by Jose Marquez, Northumbria University
13:45 – Interpreting time-resolved photoluminescence for kesterite devices and absorbers, by Charles Hages, HZB
14:05 – Effects of [Cu]/[Zn+Sn] ratio on optical spectra of CZTSe thin films on Mo/glass, by Mikhail Sulimov, Strathclyde University / Ural Federal University
14:25 – Intrinsic point defects in off-stoichiometric CZTSe kesterite type compounds, by Elisa Valle-Rios, HZB
Imec 5: Lounge 15:15 Session 4 – Progress in heterojunction formation Chair = Johan Lauwaert, Ghent University Imec 5: Room 2A 15:15 – Interface engineering of CZTSSe/CdS hetero-junction by epitaxial Al(OH) 3
15:35 – ZTO buffer layer and low temperature post annealing resulting in a 9.0 % efficient Cd-free CZTS solar cell, by Tove Ericson, Uppsala University
15:55 – Lattice-matched CZTS/CeO 2 solar cell with open circuit voltage boost, by Andrea Crovetto, Technical University of Denmark
16:15 – Evaporated CdIn 2 S 4 buffer layer for kesterite solar cells, by Leo Choubrac, IMN
Imec Cafetaria
Imec Cafetaria 19:30 End poster session, start dinner Imec Cafetaria 21:30 End of day 1
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th 09:00 Invited talk Chair = Maarja Grossberg, Tallinn University of Technology Imec Cafetaria: -1A 09:00 – Optimizing Cu-based chalcopyrites for photovoltaics - results from DFT calculations, by Clas Persson, Oslo University
09:30 – Functionalized transparent conductive oxides as back contact for kesterite solar cells, by Moises Espindola-Rodriguez, IREC
09:50 – Flexible and light-weight CZTSe solar cells fabricated at low- temperature on polymer substrate, by Edgardo Saucedo, IREC
10:10 – Improvement of V OC in kesterite solar cells by introducing metal oxide layers at rear interface and p-n junction, by Samaneh Ranjbar, imec 10:30 Coffee break – Working Groups 1 and 2 Coffee break – Working Group 3 Imec 5: Lounge Imec Cafetaria: -1A
Imec 5: Room 1A 11:00 – CZTSe surface composition and defect concentration analysis by innovative UV Resonant Raman spectroscopy, by Victor Izquierdo-Roca, IREC
11:15 – Influence of Cu content on changes in band gap energy in CZTSSe solar cell absorbers for different degrees of order, by Mario Lang, KIT
11:30 – Discussion 12:15 – Summary Working Group 2 – Progress in absorber formation Moderators = Guy Brammertz, imec & Edgardo Saucedo, IREC Imec 5: Room 1B 11:00 – Strategies for band gap graded kesterite absorbers through cation substitution, by Markus Neuschitzer, IREC
11:15 – Inclusion of alkali elements in CZTSe absorbers and their influence on physical and optoelectronic properties, by Sylvester Sahayaraj, imec
11:30 – Discussion 12:15 – Summary Working Group 3 – Progress in cell architecture Moderators = Alex Redinger, HZB & Tove Ericson, Uppsala University Imec Cafetaria: -1A 11:00 – Alternative buffers and partial electrolyte treatments for CZTSe solar cells, by Christian Andres, Empa
11:15 – Intermixing at the In x S
/CZTSSe interface and its impact on the chemical and electronic structure, by Dirk Hauschild, KIT 11:30 – Discussion 12:15 – Summary 12:30 Lunch break Imec 5: Lounge 13:30 Closing session Imec Cafetaria: -1A 13:30 – Overview of sessions 1 to 5 by Bart Vermang, imec 13:40 – Overview of working group 1 by Thomas Unold, HZB & Leo Choubrac, IMN
13:50 – Overview of working group 2 by Guy Brammertz, imec & Edgardo Saucedo, IREC
14:00 – Overview of working group 3 by Alex Redinger, HZB & Tove Ericson, Uppsala University
14:10 – Presentation of STARCELL by Edgardo Saucedo, IREC
14:20 – Discussion next workshop host by ALL 14:30 End of the Workshop (A lab visit is possible) 5
th 1 P. Balaz Stannite and its big brother kesterite: possible solid-state synthesis of both quaternary nanocrystals in scalable amounts
Materials modelling of CZTS: electrons, phonons and disorder 3 T. Raadik Low temperature time resolved photoluminescence in ordered and disordered CZTS single crystals
Structural characterisation of CZTGSe by neutron diffraction 5 G. Gurieva Investigation of detection limits of ZnSe and Cu 2 SnSe
3 secondary phases in CTZSe 6 M. Sulimov A PL and PLE study of CZTSe/Mo and ZnO/CdS/CZTSe/Mo on glass substrates 7 C. Schnohr Local kesterite composition and secondary phases in off-stoichiometric CZTSe 8 N. Ross Selenium annealing study of compound sputtered CZTS precursors 9 W. Kogler Ge-alloyed CZTGSSe solar cells with CdS and In 2 S
buffer layer 10 H. Kavak Investigation of solvent/stabilizer ratio and thermal treatment effect on CZTS absorber layer
In-situ Investigation of the order-disorder transition in CZTSe by optical transmission spectroscopy
Electrical and physical characterizations for CZTS monograin layer solar cells and modules
CZGSSe absorber formation studied by soft and hard x-ray photoelectron spectroscopy: Impact of precursor composition
A multiple-selenization process for enhanced reproducibility of CZTSSe solar cells 15 C. Rein Synthetic kesterites from deep eutectic solvents 16 A. Aziz Suzon Green annealing route for sequential processed CZTS solar cell 17 E. Saucedo Epitaxial relationships and structural quality of the CZTSe/CdS hetero-junction on the nanoscale
Spatial distribution of sodium in CZTSSe studied with secondary ion mass spectrometry image depth profiling
Annealing effect on CZTS solar cell 20 M. Valentini Stoichiometry effect on the order-disorder related E g changes in CZTS 21 M. Sayed Influence of deposition parameters on the properties of kesterite thin films prepared by spray pyrolysis
Potential fluctuations on CZTSSe solar cells admittance 23 G. Larramona Preliminary ageing tests on 11.5% CZTSSe devices spray coated from a water- ethanol ink 24 V. Kosyak The effect of sulfur vacancy concentration on the equilibrium of native point defects in CZTS
Influence of surface treatments on kesterite and CIGSe absorbers studied with Kelvin Probe force microscopy
Al 2 O 3 front surface passivation of kesterite solar cells 27 T. Schwarz Formation of nano-sized Cu-Sn-Se particles in CZTSe thin-films and their effect on solar cell efficiency
Photoluminescence in the kesterite Ag:CZTSSe absorbers with varied Ag content 29 R. Gunder Cation distribution and point defect concentration in off-stoichiometric CZGSe compound semiconductors
Investigation of the growth of CZTS nanocrystals from hot-injection synthesis
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